Personal and professional correspondence, including 25 long letters from Professor Henry F. Herbig; manuscripts (mainly speeches); specifications for patents in electrical fields; technical and personal photographs; and memorabilia. Included is a copy of the famous "shot in hand" x-ray photograph, ca. 1896, one of the first ever to be taken. This collection also contains the correspondence, manuscripts, documents, and memorabilia of Professor Pupin's daughter, Varvara Smith, and his son-in-law, Louis Graham Smith. His daughter's letters and documents deal with her financial difficulties, her administration of Pupin's estate and her claims against Columbia University. Louis G. Smith's letters deal with his anti-Communist sentiments and his manuscripts are mainly ideas for popular songs and plays. There are three letters (photostatic copies) to Smith from Dwight D. Eisenhower.

The V. K. Wellington Koo papers document the diplomatic legacy of Wellington Koo as a Chinese statesman and diplomat of the 20th Century. The papers primarily consist of materials collected during Koo's diplomatic career, relating to the Lytton Commission, 1932-1933; the League of Nations, 1931-1940; the United Nations, 1944-1946; his ambassadorships to France, 1932-1941; to Britain, 1941-1946; to the United States, 1946-1956; as the Senior Advisor to the Republic of China from 1956; and as the Judge on the International Court of Justice, 1957-1966. The materials include correspondence, diaries, memoranda, manuscripts, documents, notes, speeches, maps, photographs, printed material, and audio visual material. The bulk of the materials emphasizes China's domestic and foreign affairs, such as the Sino-Japanese conflict, World War II and the Cold War in the Far East region, as well as the League of Nations and the United Nations.