The papers include correspondence, manuscripts, and printed materials. Correspondence consists of letters from a number of important cultural figures in the emigration, including: Ivan Bunin, Zinaida Guppius, Aleksandr Kuprin, Pavel Mili︠u︡kov, Alekseĭ Remizov, Nadezhda Teffi, and Alekseĭ Tolstoĭ; there are also one or two letters each from Konstantin Balḿont, Dmitriĭ Merezhkovskiĭ, Ili︠́a︡ Repin, Fedor Shali︠a︡pin, and Marina T︠S︡vetaeva. There are manuscripts of several works by Shpoli︠a︡nskiĭ, including his memoirs, "Poezd na tretém puti" (New York, 1954).

The collection consists of correspondence, manuscripts, documents, a photograph, and printed material, primarily from the period 1941-1957. Included are letters from Ivan Bunin, Marc Chagall, Mikhail Karpovich, Vasiliĭ Maklakov, W. Somerset Maugham, Vladimir Nabokov, Ili︠́a︡ Repin, Edmund Wilson, Boris Zaĭt︠s︡ev and many others. Manuscripts of his works include "Istoki""Nachalo kont︠s︡a""Zhivi, kak khochesh"́, and "The Escape" (English translation of "Begstvo"), such shorter tales as "Noch ́v terminale""Povest ́o smerti", and "Ulḿskai︠a︡ noch"́, as well as numerous articles, book reviews and essays. There are financial records for "Novyĭ Zhurnal", which Aldanov helped found, and the clippings are mainly articles about Aldanov. There is one late photograph of Aldanov.