The Chen Lifu papers (陳立夫檔案) mainly document his involvement in Chinese politics during the Republican era, dating from 1926 to 1989, with the bulk dates from 1926 to 1951. The papers consist of correspondence, portrait, meeting documents, reports, plans, speeches, writings, memoir, and printed materials. The papers focus on Chen Lifu's political career as the Head of the Central Bureau of Investigation and Statistics and the Minister of Education, as well as his general involvement in politics dating from 1926 to 1949.

The Chinese oral history project collection (中國口述歷史項目檔案) provides a wealth of information on the development of the project and its interviews with eminent Chinese political figures abroad in the United States and Hong Kong from 1958 to 1980s. The highlights of the collection consist of the administrative subject files, correspondence, interview photographs and reports, transcript drafts, collected autobiographies and manuscripts, audio recordings, and card files of names mentioned in the transcripts.