The collection consists mainly of correspondence, financial records, and subject files. Also included are protocols of meetings and reports, photographs, membership and subscription lists, and printed materials. The cataloged materials include manuscripts sent by such authors as Alekseĭ Remizov and Boris Zaĭt︠s︡ev for "Den ́Russkogo Rebenka" (Day of the Russian Child) in the 1930s, as well as correspondence from Nikolaĭ Vakar, Claire Boothe Luce, Aleksandra Tolstai︠a︡, and others. The bulk of the collection consists of correspondence with and about beneficiaries, and financial records from the period 1926-57.

Correspondence, manuscripts, notes, documents, photographs and printed materials of Frank. The collection reflects almost every aspect of his career, but especially his life in Germany, France, and England after his expulsion from Russia in 1922. Among the correspondents are Nikolaĭ Berdi︠a︡ev, Sergeĭ Bulgakov, Albert Einstein, Georgiĭ Florovskiĭ, Nikolaĭ Losskiĭ, Fedor Stepun, and Petr Struve; there are one or two items each from Vi︠a︡cheslav Ivanov, Bernard Pares, and Alekseĭ Remizov. There are also many letters from Semen Frank and his wife Tati︠a︡na to their son Viktor, and from Peter Struve's family to the Franks. Manuscripts for several of Frank's books are in the collection, such as "Svet vo tḿe" "Realńost ́i chelovek" and "Biografii︠a︡ P.B. Struve." Other manuscript materials by Frank include essays and lectures, outlines of courses he taught as a professor in Russia before his expulsion, and notebooks. There are also two poems by Vi︠a︡cheslav Ivanov. Among the printed works are Frank's Bible and offprints of his articles. There are photographs of Sergeĭ Bulgakov, Fedor Stepun, and of the Frank and Struve families.

Correspondence, manuscripts, documents, photographs, subject files, and printed materials of members of the Zernov family, especially Nikolaĭ M. Zernov. Correspondence includes letters from Nikolaĭ Berdi︠a︡ev, Archimandrite Kiprian, Alekseĭ Remizov, Vasiliĭ Zenḱovskiĭ, and copies of many letters from Gustave Kullmann to his wife Marii︠a︡, nʹee Zernova. Manuscripts include: memoirs by Sofii︠a︡ A. Zernova about her childhood, youth, and family; Sofii︠a︡ M. Zernova's albums, poems, diaries and memoirs about the Civil War and the emigration in Europe; manuscripts by Nikolaĭ Zernov on religious and literary themes; a report by a Lt. Shokotov on his White Army detached service in 1917-1919; a brief manuscript by Vladimir M. Zernov claiming that syphillis was a contributing factor in Lenin's death; and manuscripts and speeches by Kullmann. Subject files include biographical information collected by Nikolaĭ Zernov on many emigre Orthodox churchmen and religious writers, and materials relating to Kullmann and the Zernov family.